For the Hash:
Place potatoes in a 3-quart saucepan and cover with 2 quarts cold water. Add vinegar and 2 tablespoons kosher salt. Bring to a boil over high heat. Reduce to a simmer and cook until barely tender, about 7 minutes after coming to a boil. Drain potatoes in a colander, then set aside. Meanwhile, heat a large cast iron skillet over high heat for 5 minutes. Add asparagus and serrano to the pan and arrange in a single layer. Cook, turning occasionally until asparagus and serrano are charred all over and asparagus is just cooked through, 4 to 6 minutes for thin spears, 5 to 8 minutes for thick spears. Carefully add 1 teaspoon pork fat to the skillet, toss to coat vegetables, and season lightly with salt and pepper. Transfer vegetables to cutting board.
Wipe out skillet, return it to stovetop, and lower heat to medium. Add 1 tablespoon plus 2 teaspoons pork fat and pulled roast pork shoulder to now-empty skillet, and arrange pork in a single layer. Season lightly with salt and pepper, and cook, stirring occasionally, until pork is golden brown and crisp on all sides, 8 to 10 minutes. Using a slotted spoon, transfer pork to a plate and set aside.
Add remaining 2 tablespoons pork fat to skillet and increase heat to medium-high. Add potatoes and arrange in as even a single layer as possible. Season lightly with salt, and cook, stirring and tossing occasionally, until potatoes are deep brown and crisp on all sides, about 20 minutes. Add coriander, chili powder, and cumin and cook, stirring frequently, until fragrant, about 30 seconds.
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